wii can do n64 full speed which is a more powerful console then the ps1
in the world of electronics 1+1 doesn't always equals 2.
the wii can do n64 full speed on select games because nintendo engineered an emulator and tweaked it so it can run those specific titles.
the raspberry pi 3 is more powerful than a wii in raw numbers but it doesn't have the level of software optimization to achieve good n64 emulation, but still the rpi3 is powerful enough to run select games at full speed with minimal glitches.
now the thing about ps1 emulation is that pcsx-rearmed has a heavily optimized (for arm with neon) dynarec core while the wii can't run pcsx-rearmed because it uses a completely different cpu architecture. something similar goes for the 3ds, it has an arm cpu but lacks neon support.
I am going to quote tom here because he generally has everything laid out in a way that is easy to understand. I suggest the Pi 3 even if some of the bigger games are kinda laggy. I have a Pi 3 running some PS1 games and it really works well. I played some THPS2 just the other night with little to no issues.
what heavy games are we talking about here?
I have played metal gear solid completely lag free and with all the visual effects intact, considering that mgs is very intensive with its frame buffer usage I would say that every game should play perfectly fine save a few exceptions. in fact, the only exception that I have seen is sheep raider that has slowdowns in specific situations (if you are curious, leave the demo play the 2 levels it shows).
all with stock settings for pcsx-rearmed.
EDIT: oh and I guess the main menu of soul blade too, is very intensive and lags for some reason, on my laptop with mednafen I even have to put the high performance profile to run that menu without lagging.