The 18+ ones which I recommend:
Tsukihime
Fate/stay Night (Filesize for the version with sound is pretty big, may take time to load)
Saya no Uta (Warning: not for the weak of heart)
As for the non 18+ ones, True Remembrance has a great story for a non-commercial visual novel. Red Shift is a good one too, but the ending's kind of cheesy, haha. Try Narcissu too, though I personally think this one is better on the computer. Actually, most of the ported visual novels for VNDS are pretty good. Anyway, the ones I really recommend for non 18+:
True Remembrance
Red Shift
Narcissu
Tegami/The Letter
Plain Song
Out of all of these, the best in terms of story is probably Tsukihime and Fate/stay Night. Hope this helps.
I don't know if it'll work for you: But the PC game "Dividead" is AWESOME! it's 18+ though.... but even if you'd pick all the 18+ scenes out, it'd be a great game!
Of course, there's also the ported visual novels at VNDS three of which are not freeware (Tsukihime, Fate/stay Night, Saya no Uta)... which can be found here.
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