I have some easy and obvious answers for you.
Elfen Lied
Akira
Vampire Hunter D I & II
Ninja Scroll (original movie not series)
Blood (original movie not series)
Metropolis (not the silent film from 1927, but that is AWESOME TOO!)
Coonskin
Fire and Ice
Fritz the Cat
Heavy Traffic
Hey Good Lookin
The Nine Lives of Fritz the Cat
Wizards
American Pop
Lord of the Rings (also don't forget Lord of the Rings Completely Screwed Over "on youtube)
Adventures of Mark Twain
Classic Warner Brothers and anything by Chuck Jones
G.I. Joe Resolute
Gandahar
Heavy Metal
Samurai Jack
Shinbone Alley
Classic Don Bluth Disney
Starchaser: The Legend of Orin
The Iron Giant
The Secret of Nihm
The Castle of Cagliostro
Time Masters
When the Wind Blows
Who Framed Roger Rabbit
Water Ship Down
Plague Dogs
Grave of the Fireflies
Green Legend Ran
Nausicaa
My Neighbour Totoro
Mary and Max
Mike Judge Presents: The Animation Show
Les Escargots
Pinochhio & The Emperor of the Night
She and Her Cat
Ys Legacy
Fist of the North Star (movie)
Jack and the Beanstalk
Wall-E
Toy Story Trilogy
William S.Burroughs - The Junky's Christmas
The Railway Dragon
The Maxx
The Care Bears Movie
Berserk
Twice Upon a Time
The Mouse and His Child
The Phantom Tollbooth
The Watchmen Motion Comic
Superman - Red Sun motion comic.
Doggy Poo
Batman The Animated Series (early 90's)
Princess Monoke
Ghost in the Shell (original movie)
And here is the list to prove beyond proof that most of today's cartoons just ain't got now soul!
"The care bears movie" Thanks, just what I was looking for