In theory you can run RetroArch. I've tried to build it a while ago and it didn't work, the way the device uses SDL is not trivial for a noob like me.Can you run Retroarch on this, and has anyone tried the Legend Flashback UI with this, most all Atgames Flashbacks use the same UI, look at Atari Flashback 9 and X..?
Is there a post about how to connect this to a UART and Putty..?
Changing the UI with the Legends Flashback means you will lose access to the cartridge port, so it might not worth it.
Connecting to the UART is simple on the pinout perspective (I don't recall the order, but it's basically RX, TX and GND), but you need a UART adapter supporting 1500000 baud, which most doesn't support. There are lots of guides on how to connect a SBC, it's the same process.